Wet deposition

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NOTE: Page under construction!

This page describes the current wet deposition scheme used in GEOS-Chem.

Overview

The Harvard Atmospheric Chemistry Modeling Group developed a wet deposition scheme for the GMI model, and then implemented it into GEOS-Chem. Jacob et al 2000 describes the algorithm in full.

The wet deposition scheme includes scavenging of soluble tracer in convective updrafts, as well as rainout and washout of soluble tracers.

Validation

Text to be added

References

  1. Domine, F., and E. Thibert, Mechanism of incorporation of trace gases in ice grown from the gas phase, Geophys. Res. Lett., 23, 3627-3630, 1996.
  2. Giorgi, F., and W.L. Chameides, Rainout lifetimes of highly soluble aerosols as inferred from simulations with a general circulation model, J. Geophys. Res., 91, 14,367-14,376, 1986.
  3. Jacob, D.J., Heterogeneous chemistry and tropospheric ozone, Atmos. Environ., 34, 2131-2159, 2000. PDF
  4. Jacob, D.J. H. Liu, C.Mari, and R.M. Yantosca, Harvard wet deposition scheme for GMI, Harvard University Atmospheric Chemistry Modeling Group, revised March 2000. PDF
  5. Levine, S.Z., and S.E. Schwartz, In-cloud and below-cloud scavenging of nitric acid vapor, Atmos. Environ., 16, 1725-1734, 1982.
  6. Liu, H., D.J. Jacob, I. Bey, and R.M. Yantosca, Constraints from 210Pb and 7Be on wet deposition and transport in a global three-dimensional chemical tracer model driven by assimilated meteorological fields, J. Geophys. Res., 106, 12,109-12,128, 2001. PDF
  7. Mari, C., D.J. Jacob, and P. Bechtold, Transport and scavenging of soluble gases in a deep convective cloud, J. Geophys. Res., 105, 22,255-22,267, 2000. PDF
  8. Selin, N.E. and D.J. Jacob, Seasonal and spatial patterns of mercury wet deposition in the United States: North American vs. intercontinental sources, Atmospheric Environment, 42, 5193-5204, 2008. PDF

Known issues

Negative tracer in routine WETDEP because of negative RH

See this post: GEOS-5 issues#Small negative RH value in 20060206.a6.2x25 file

Fixes are available at ftp://ftp.as.harvard.edu/pub/geos-chem/patches/v8-01-01.

--phs 16:31, 6 June 2008 (EDT)

Negative tracer in routine WETDEP

Dylan Millet wrote:

I'm having a run die consistently at the same time (October 1, 2005; first time step of the month) in large-scale wetdep, with an STT element < 0.
  • Platform: Linux cluster
  • Threads: 8
  • Version: v7-4-13 out of the box.
  • GEOS4, 4x5, 30L, full chemistry
  • IFORT 10.1
In Section 6 (No Downward Precip) of wetscav_mod.f, subroutine safety is getting called.
    WETDEP - STT < 0 at    1   1  29 for tracer    7 in area    6
(First of all it seems odd to do wetdep for L=29, this is 63 km up). Have you seen anything like this? I ran for the whole year starting Jan 1 successfully until this point.
... By the way, the problem persists when I turn off chemistry altogether.

Philippe Le Sager replied:

I used your restart file and the same input.geos (w/ chemistry on and off). My code went thru without problem. I tried both Sun Studio and Ifort 9 compilers, and the later on two different machines (altix and ceres). I used v7-04-13 and v8-01-01. I never reproduced your error.
We just got the new Ifort 10, and tried it too. I run v8-01-01 without an error. But when I tried v7-04-13, I finally reproduced your error, with the exact same negative values!
In other words: the bug happens with IFort 10 and v7-04-13 only.
Also, have a look at this recent development. This is not the reason for your bug (I tried v8 w/ ifort 10 and isorropia -like v7-04-13- and it did not crash), but using RPMARES instead of Isorropia may be a way to fix it.
... More about the Ifort 10 / v7-04-13 issue. When I wanted to debug with TotalView, I could not reproduce the bug anymore.... because I simply suppress any optimization. So, I did more test and found that if the default -O2 optimization is used, GEOS-Chem crashes. But it works fine with -O1. It is hard to tell what happens, since only the emissions step is done between reading the restart file and the crash.
Bob and I will further test Ifort 10 for optimization on our machines. Maybe we will find something... For the time being, you may have to switch to -O1, at least for the run that crashes. You will find the optimization flag at the beginning of the Makefile.ifort.

Long story short: This appears to be an optimization issue with IFORT 10 and v7-04-13. Upgrading to GEOS-Chem v8-01-01 should solve this problem.

--Bmy 10:38, 17 April 2008 (EDT)